| Ambient concentrations and deposition rates of selected reactive nitrogen species and their contribution to PM2.5 aerosols at three locations with contrasting land use in southwest China | |
Song, Ling1,2 ; Liu, Xuejun3; Skiba, Ute4; Zhu, Bo1,2; Zhang, Xifeng1,2; Liu, Meiyu2; Twigg, Marsailidh4; Shen, Jianlin5; Dore, Anthony4; Reis, Stefan4; Coyle, Mhairi4; Zhang, Wen3; Levy, Peter4; Fowler, David4
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| 2018-02-01 | |
| Source Publication | ENVIRONMENTAL POLLUTION
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| ISSN | 0269-7491 |
| Volume | 233Pages:1164-1176 |
| Abstract | The fast economic development of southwest China has resulted in significant increases in the concentrations of reactive nitrogen (Nr) in the atmosphere. In this study, an urban (Chengdu, CD), suburban (Shifang, SF) and agriculture (Yanting, YT) - dominated location in the Sichuan Province, southwest China, were selected to investigate the atmospheric composition of Nr, their concentrations and deposition rates. We measured Nr concentrations in precipitation (NH4+, NO3- and organic N (DON)), the gas phase (NH3 and NO2), and the aerosol particles (PM2.5), and calculated their fluxes over a two year period (2014-2016). Total annual N deposition rates were 49.2, 44.7 and 19.8 kg N ha(-1) yr(-1) at CD, SF and YT, respectively. Ammonia concentrations were larger at the urban and suburban sites than the agricultural site (12.2, 14.9, and 4.9 mu g N m(-3) at CD, SF and YT, respectively). This is consistent with the multitude of larger sources of NH3, including city garbage, livestock and traffic, in the urban and suburban areas. Monthly NO2 concentrations were lower in warmer compared to the colder months, but seasonal differences were insignificant. Daily PM2.5 concentrations ranged from 7.7 to 236.0, 5.0-210.4 and 4.2 -128.4 mu g m(-3) at CD, SF and YT, respectively, and showed significant correlations with fine particulate NH4+ and NO3- concentrations. Ratios of reduced to oxidized N were in the range of 1.6-2.7. This implies that the control of reduced Nr especially in urban environments is needed to improve local air quality. (C) 2017 Elsevier Ltd. All rights reserved. |
| Keyword | Reduced nitrogen Oxidized nitrogen Seasonal pattern Pollution source Land use type |
| DOI | 10.1016/j.envpol.2017.10.002 |
| WOS Keyword | CENTRAL SICHUAN BASIN ; DRY DEPOSITION ; ATMOSPHERIC AMMONIA ; INORGANIC NITROGEN ; SULFUR-DIOXIDE ; AIR-QUALITY ; CHEMICAL CHARACTERISTICS ; TRANSPORT MODELS ; RURAL SITES ; EMISSIONS |
| Language | 英语 |
| Funding Project | Natural Science Foundation of China[41301321] ; Natural Science Foundation of China[41271321] ; Natural Science Foundation of China[41371303] ; Major Science and Technology Program for Water Pollution Control and Treatment[2017ZX07101-001] ; Chinese Academy of Sciences (light of West China' Program) ; CINAg project |
| WOS Research Area | Environmental Sciences & Ecology |
| WOS Subject | Environmental Sciences |
| WOS ID | WOS:000424177000124 |
| Funding Organization | Natural Science Foundation of China ; Major Science and Technology Program for Water Pollution Control and Treatment ; Chinese Academy of Sciences (light of West China' Program) ; CINAg project |
| Publisher | ELSEVIER SCI LTD |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.imde.ac.cn/handle/131551/20648 |
| Collection | 山地表生过程与生态调控重点实验室 综合测试与模拟中心 |
| Corresponding Author | Zhu, Bo |
| Affiliation | 1.Chinese Acad Sci, Key Lab Mt Surface Proc & Ecol Regulat, Chengdu 610041, Sichuan, Peoples R China 2.Chinese Acad Sci, Inst Mt Hazards & Environm, Chengdu 610041, Sichuan, Peoples R China 3.China Agr Univ, Coll Resources & Environm Sci, Beijing 100193, Peoples R China 4.Ctr Ecol & Hydrol, Bush Estate, Penicuik E1126 0QB, Midlothian, Scotland 5.Chinese Acad Sci, Inst Subtrop Agr, Key Lab Agroecol Proc Subtrop Reg, Changsha 410125, Hunan, Peoples R China |
| First Author Affilication | 中国科学院水利部成都山地灾害与环境研究所 |
| Corresponding Author Affilication | 中国科学院水利部成都山地灾害与环境研究所 |
| Recommended Citation GB/T 7714 | Song, Ling,Liu, Xuejun,Skiba, Ute,et al. Ambient concentrations and deposition rates of selected reactive nitrogen species and their contribution to PM2.5 aerosols at three locations with contrasting land use in southwest China[J]. ENVIRONMENTAL POLLUTION,2018,233:1164-1176. |
| APA | Song, Ling.,Liu, Xuejun.,Skiba, Ute.,Zhu, Bo.,Zhang, Xifeng.,...&Fowler, David.(2018).Ambient concentrations and deposition rates of selected reactive nitrogen species and their contribution to PM2.5 aerosols at three locations with contrasting land use in southwest China.ENVIRONMENTAL POLLUTION,233,1164-1176. |
| MLA | Song, Ling,et al."Ambient concentrations and deposition rates of selected reactive nitrogen species and their contribution to PM2.5 aerosols at three locations with contrasting land use in southwest China".ENVIRONMENTAL POLLUTION 233(2018):1164-1176. |
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